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Journal Articles

High quality single crystal growth of a novel superconductor UTe$$_2$$; Improvement of $$T_{rm c}$$ and multiple superconducting phase diagram

Sakai, Hironori; Haga, Yoshinori

Kotai Butsuri, 58(10), p.529 - 536, 2023/10

We have succeeded to grow high-quality UTe$$_2$$ single crystals with excess uranium through molten salt flux method. We have also studied the superconducting phase diagram using the high-quality crystal applying the fields up to 25 T along the magnetic hard $$b$$ axis.

Journal Articles

Single crystal growth of superconducting UTe$$_2$$ by molten salt flux method

Sakai, Hironori; Opletal, P.; Tokiwa, Yoshifumi; Yamamoto, Etsuji; Tokunaga, Yo; Kambe, Shinsaku; Haga, Yoshinori

Physical Review Materials (Internet), 6(7), p.073401_1 - 073401_10, 2022/07

 Times Cited Count:18 Percentile:89.58(Materials Science, Multidisciplinary)

The molten salt flux method is applied as a new synthetic route for the single crystals of the spin-triplet superconductor UTe$$_2$$. The single crystals under an optimized growth condition with excess uranium exhibit a superconducting transition at $$T_{rm c}=2.1$$ K, which is the highest $$T_{rm c}$$ reported for this compound. The obtained crystals show a remarkably large residual resistivity ratio with respect to the room temperature value and a small residual electronic contribution in specific heat well below $$T_{rm c}$$. These results indicate that the increase of $$T_{rm c}$$ in UTe$$_2$$ can be achieved by reducing the disorder associated with uranium vacancies. The excess uranium in the molten salt acts as a reducing agent, preventing tetravalent uranium from becoming pentavalent and suppressing creation of uranium vacancies. At the same time, the relatively low growth temperature can suppress Te volatilization.

Journal Articles

The dHvA experiment under pressure in UIr

Shishido, Hiroaki*; Yamamoto, Etsuji; Haga, Yoshinori; Ikeda, Shugo; Nakashima, Miho*; Settai, Rikio*; Onuki, Yoshichika

Journal of the Physical Society of Japan, 75(Suppl.), p.119 - 120, 2006/08

 Times Cited Count:1 Percentile:11.01(Physics, Multidisciplinary)

no abstracts in English

Journal Articles

Pure single crystal growth and odd parity superconductivity in UPt$$_{3}$$

Onuki, Yoshichika*; Yamamoto, Etsuji; Haga, Yoshinori; Kimura, Noriaki*

Genshiryoku Kogyo, 43(5), p.47 - 52, 1997/00

no abstracts in English

Oral presentation

Single crystal growth and superconducting properties of novel superconductor UTe$$_2$$

Sakai, Hironori

no journal, , 

I will present the recently developed method for growing high-quality single crystals of UTe$$_2$$ and report the superconducting properties by these crystals.

Oral presentation

Multiple superconducting phases in the novel superconductor UTe$$_2$$ revealed by high-quality single-crystal

Sakai, Hironori

no journal, , 

We have recently succeeded in growing ultra-clean single crystals of the novel superconductor UTe$$_2$$ using the molten salt flux (MSF) method, which increases $$T_{rm c}$$ from 1.6 K to 2.1 K by suppressing impurity scattering. When a magnetic field is applied "precisely" in the magnetization-hard b-axis direction, a "field-enhanced superconducting state" appears, in which $$T_{rm c}$$ increases with the magnetic field above 15 T. To investigate this high-field superconducting (HFSC) phase, we attempted to determine the field-temperature phase diagram of ultra-pure single crystals up to $$sim$$25 T. With applying magnetic field along the $$b$$-axis, the simultaneous measurements of $$rho$$ and $$Deltachi_{rm AC}$$ revealed an intermediate superconductivity between the low-field superconducting (LFSC) and HFSC phases above $$sim$$15 T, previously hidden in the low-quality samples.

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